1 Double-Resonance Spectroscopy.- 1.1. Introduction to Double-Resonance Methods.- 1.2. Response of a System to Pumping and Analyzing Radiation Fields.- 1.3. Experimental Considerations.- 1.4. Microwave-Detected Double Resonance.- 1.5 Infrared-Detected Double Resonance.- 1.6. Optically Detected Double Resonance.- 1.7. Molecular Information from Double-Resonance Experiments.- References.- 2 Coherent Transient Microwave Spectroscopy and Fourier Transform Methods.- 2.1. Introduction.- 2.2. Basic Theory and Experiment.- 2.3. ...
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1 Double-Resonance Spectroscopy.- 1.1. Introduction to Double-Resonance Methods.- 1.2. Response of a System to Pumping and Analyzing Radiation Fields.- 1.3. Experimental Considerations.- 1.4. Microwave-Detected Double Resonance.- 1.5 Infrared-Detected Double Resonance.- 1.6. Optically Detected Double Resonance.- 1.7. Molecular Information from Double-Resonance Experiments.- References.- 2 Coherent Transient Microwave Spectroscopy and Fourier Transform Methods.- 2.1. Introduction.- 2.2. Basic Theory and Experiment.- 2.3. Transient Absorption.- 2.4. Transient Emission.- 2.5. Fast Passage.- 2.6. Fourier Transform Microwave Spectroscopy.- 2.7. Molecular Interpretation of T1 and T2.- 2.8. Conclusion.- Appendix A. Solution of the Bloch Equations.- Appendix B. Two-State Relaxation Processes.- References.- 3 Coherent Transient Infrared Spectroscopy.- 3.1. Introduction.- 3.2. Density and Population Matrices.- 3.3. Absorption and Emission of Radiation.- 3.4. Solutions of the Population Matrix Equations.- 3.5. Experimental Techniques.- 3.6. Optical Nutation.- 3.7. Optical Free Induction Decay.- 3.8. Photon Echo.- 3.9. Measurement of Level Decay Rates.- 3.10. Velocity-Changing Collisions.- Appendix A. Justification of the Reduced Wave Equation.- Appendix B. Matrix Formulation of the Bloch Equations.- References.- 4 Coherent Spectroscopy in Electronically Excited States.- 4.1. Introduction.- 4.2. Theoretical Considerations.- 4.3. Experimental Methods.- 4.4. Applications.- References.- 5 Resonant Scattering of Light by Molecules: Time-Dependent and Coherent Effects.- 5.1. Elementary Time-Dependent Theory Related to Luminescence.- 5.2. Applications of Scattering Theory to Model Systems.- 5.3. Nature of the Electromagnetic Field.- 5.4. Theory of Light Scattering with Well-Defined LightSources.- 5.5. Effects of Intermolecular Interactions on Luminescence.- 5.6. Two-Photon Induced Light Scattering.- 5.7. Recent Resonance Fluorescence Concepts and Experiments.- Appendix. Contour Integration.- References.- Author Index.
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